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FMA:B- Againg by Yui
all openings and endings from Ao no Exorcist
Fate/Stay Night opening 2
Deadman Wonderland - One Reason by Fade
Kuroshitsuji II - Shiver by The Gazette
Higurashi no naku koro ni opening and opening from umineko no naku koro ni
... and a lot more 
Opening: BLUE (Bleach)
Ending: Junketsu Paradox (Blood-C)
Almost all the InuYasha opening/endings. Do As Infinity is so AMAZING. (:
Bakusou Yumeuta-Diggy Mo'
Whats up People-Maximum the Hormone
all detective conan openings
full methal alchemist first oppening: Again by YUI
naruto opening 3, 5, 9
Naruto Shippuden: Blue Bird by Ikimono Gakari
Durarara: Uragiri no Yuuyake by THEATRE BROOK
Inuyasha: My Will, Dearest
My favorites at the moment are:
Hitori Samishiku - ShaNa ~~ Fairy Tail
kimi no shiranai monogatari - Supercell ~~ Bakemonogatari
Gekidou - UVERworld ~~ D.Gray-man
Hack/Sign: Yasashii Yoake by See Saw
Ghost In The Shell: Inner Universe and Rise By Yoko Kanno
Last Exile: Cloud Age Symphony by Shuntaro Okino and Over The Sky by Hitomi Kuroishi.
Ruorouni Kenshi: Hearts of Swords T.M.Revolution and 1/2 Kawamoto Makoto.
Fullmetal Alchemist & Brotherhood: L'Arc~en~Ciel Ready Steady Go!, YUI Again, Golden Time Lover Sukima Switch, Lie by SID, LET IT OUT by Fukuhara Miho, Tsunaida Te by Lil'B
Ghost Hound: Poltergeist by Mayumi Kojima and Call My Name by Yucca
Clannad: Dango Daikazako By Chata
East Of Eden: Futuristic Imagination by School Food Punishment
Nana: Rose and Shape of Your Love by Anna Tsuchiya
Initial D 4th Stage: Nobody Reasons by M.O.V.E
Gokudou-kun Manyuuki: プリズム (Prism) by BAISER (<- favorite song ever; I found that anime through BAISER, actually xD)
Death Note: all opening and ending themes
InuYasha (man, that show has some good songs. Ain't nothin' like an old anime. 
) - every heart., My Will, Fukai Mori and Shinjitsu no Uta (last two by D･O･A)
FMA: READY STEADY GO! by L'arc~en~Ciel
FMA:B : Again - YUI
.hack// : New World by Round Table and that one song from .hack//SIGN... I dunno the name of it... 
BLEACH: D-technolife by UVERworld
Vampire Knight: Still Doll by Kanon Wakeshima
Ghost in the Shell: Inner Universe by Yoko Kanno
Opening Songs from: La Cordia, Inuyasha, Kuroshitsuji I & II, Durarara
Ending songs from: Kuroshitsuji II, Vampire Knight, Inuyasha, Durarara
I love the "anime songs" made by "I've Sound" and "Eufonius".
From I've Sound, KOTOKO's "Agony" is one of my favorites, even not seeing the anime it come from.
From Eufonius, "Narcissus" (from doujin visual novel "Narcissu -side 2nd-") is one of my favorites.
Shunkan Sentimental by Scandal from Fullmetal Alchemist: Brotherhood
My choices would be...
Errand>>Feylan (seikon no qwaser)
Futatsu no kadou to akai tsumi>>On/Off (Vampire knight)
Rondo>>On/Off (Vampire knight 2)
Parallel hearts>>Fiction Juction (Pandora Hearts)
and much much more!!!!!
yokan- heidifrom kaichou wa maid sama
alones
sen no yoru wo koete by aqua timez from bleach.
Any opening and closing from Gundam OO! they all were perfect!
Ichiban no takaramono By Lisa - Angel Beats
kimi no shiranai monogatari By Supercell - bakemonogatari
Orange BY Rie Kugimmiya - toradora
Super Driver By aya hirano - Suzumiya
Juliet - LM.CRed Garden
The Love Song - LM.C Nago someshit someshit........
OP Alonez by Aqua Timez (Bleach)
END Alumina by Nightmare (Death Note)
Hmm,
Fictionjunction - Parallel Hearts (Pandora Hearts OP),
L'Arc En Ciel - Driver'S High (Great Teacher Onizuka OP)
Baby U! - Mblaq Beelzebub
Be as one - W-inds. Fairy Tail
Anime Openings by SID:
Monokuro No Kisseu for Kuroshitsuji seasons 1,2 and the ova series
Ranbu No Melody for Bleach opening 13
By ViViD:
Blue For Bleach opening 14
By T.M Revolution:
Resonance for Soul Eater
also for Soul Eater PAPERMOON by Tommy Heavenly6
By Abington Boys School:
Howling for Darker than Black
Innocent Sorrow for D.Gray Man
By Nami Tamaki:
Brightdown for D.Gray Man
By Cheiko Kawabe:
Sakura Kiss for O.H.S.H.C
First ending of D.Gray Man Snow Kiss by Nirgilis
Second ending of D.Gray Man Antoinette Blue by Nana Kitade
Kuroshitsusji ending I'm Alive by Bella
Needless to say I like and Luv more openings than endings
